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Abstract The detailed anisotropic dispersion of the low-temperature, low-energy magnetic excitations of the candidate spin-triplet superconductor UTe₂is revealed using inelastic neutron scattering. The magnetic excitations emerge from the Brillouin zone boundary at the high symmetryYandTpoints and disperse along the crystallographic$$\hat{b}$$ $\hat{b}$-axis. In applied magnetic fields to at leastμ₀H= 11 T along the$$\hat{c}-{\rm{axis}}$$ $\hat{c}-\mathrm{axis}$, the magnetism is found to be field-independent in the (hk0) plane. The scattering intensity is consistent with that expected from U³⁺/U⁴⁺ f-electron spins with preferential orientation along the crystallographic$$\hat{a}$$ $\hat{a}$-axis, and a fluctuating magnetic moment ofμ_eff=1.7(5)μ_B. We propose interband spin excitons arising fromf-electron hybridization as a possible origin of the magnetic excitations in UTe₂. 

Abstract Magnetic and electronic properties of quantum materials heavily rely on the crystal structure even in the same chemical compositions. In this study, it is demonstrated that a layered tetragonal EuCd 2 Sb 2 structure can be obtained by treating bulk trigonal EuCd 2 Sb 2 under high pressure (6 GPa) and high temperature (600 °C). Magnetization measurements of the newly formed layered tetragonal EuCd 2 Sb 2 confirm an antiferromagnetic ordering with Neel temperature ( T N ) around 16 K, which is significantly higher than that ( T N ≈ 7 K) of trigonal EuCd 2 Sb 2 , consistent with heat capacity measurements. Moreover, bad metal behavior is observed in the temperature dependence of the electrical resistivity and the resistivity shows a dramatic increase around the Neel temperature. Electronic structure calculations with local density approximation dynamic mean–field theory (LDA+DMFT) show that this material is strongly correlated with well‐formed large magnetic moments, due to Hund's coupling, which is known to dramatically suppress the Kondo scale.